The Secretary of the Treasury halted redemption of silver certificates for silver dollar coins in March 1964. So, I assume that you could redeem in 1963. Further, you could redeem for silver bullion up to June 1968. At least that is what the Treasury stated.
RE: Coin Shop Currency - SILVER CERTIFICATE - FIVE DOLLARS - 20180610
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Coin Shop Currency - SILVER CERTIFICATE - FIVE DOLLARS - 20180610